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Stereocontrolled Total Synthesis of (+)-Altohyrtin A/Spongistatin 1 Financial support was provided by the EPSRC (GR/L41646), Cambridge Commonwealth Trust (Scholarship to M.J.C.), EC (Marie Curie Postdoctoral Fellowship to J.L.A.), DFG (Postdoctoral Fellowship to T.T.), NSERC-Canada (Postdoctoral Fellowship to R.M.O.), Churchill College (Research Fellowship to D.J.W.), Kingapos;s College and Sims Fund, Cambridge (Scholarship to D.Y.K.C.). We also thank Merck and AstraZeneca Pharmaceuticals for generous support, and Dr. Anne Butlin (AZ) and Dr. Nick Bampos (Cambridge) for valuable assistance.
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2008
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2000
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Enzyme Inhibitors from Marine Invertebrates
2007
A synthesis of biaryls via nickel(0)-catalyzed cross-coupling reaction of chloroarenes with phenylboronic acids
1996
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2006
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2006
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2010
A new approach to the synthesis of functionalized pyrido[2,3-b]indoles by way of a palladium-catalyzed ring closing reaction between the N-1 and C-9a positions
1998
First Suzuki–Miyaura type cross-coupling of ortho-azidobromobenzene with arylboronic acids and its application to the synthesis of fused aromatic indole-heterocycles
2007
The Chemistry and Biochemistry of Vanadium and the Biological Activities Exerted by Vanadium Compounds
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A three-component coupling approach to the marine bis-indole alkaloids: Topsentin, deoxytopsentin and bromotopsentin
1996
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2006
Aerobic Copper-Catalyzed Organic Reactions
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2007
Synthesis of Trithiolanes and Tetrathianes from Thiiranes Catalyzed by Ruthenium Salen Nitrosyl Complexes
2002
Promotion of IL-8 production in PMA-stimulated HL-60 cells by sesquiterpene quinones from a marine sponge, Hippospongia sp.
2007
Artificial Organic Host Molecules for Anions
1997 Standout
Mimicking Polyolefin Carbocyclization Reactions: Gold-Catalyzed Intramolecular Phenoxycyclization of 1,5-Enynes
2009
Metalated Heterocycles and Their Applications in Synthetic Organic Chemistry
2004
β-Carboline Alkaloids from a Korean Tunicate Eudistoma sp.
2008
Bioactive Sesterterpenes and Triterpenes from Marine Sponges: Occurrence and Pharmacological Significance
2010
Halogenated Compounds from Marine Algae
2010
Botryllamides A-D, new brominated tyrosine derivatives from styelid ascidians of the genus Botryllus
1995
Reversal of Diastereoselectivity of Nitrile Oxide 1,3-Dipolar Cycloadditions by Mg(II). Acceleration of Cycloaddition by Microwave Irradiation
2000
Functional Oligothiophenes: Molecular Design for Multidimensional Nanoarchitectures and Their Applications
2009 Standout
Cytotoxic bromoditerpenes from the red alga Sphaerococcus coronopifolius
2008
Biological activities of marine sesquiterpenoid quinones: structure–activity relationships in cytotoxic and hemolytic assays
2004
A Cyclized Didemnimide Alkaloid from the Caribbean Ascidian Didemnum conchyliatum
1998
Magnetically Recoverable Nanocatalysts
2011 Standout
Large-Scale Applications of Transition Metal-Catalyzed Couplings for the Synthesis of Pharmaceuticals
2011 Standout
A short route to functionalized imidazo[4,5- c ]carbazoles. Synthesis of the first example of the imidazo[4,5- c ]β-carboline ring system
2001
Cytotoxic Terpene Quinones from Marine Sponges
2010
Leptoclinidamines A−C, Indole Alkaloids from the Australian Ascidian Leptoclinides durus
2009
Advances in Synthetic Applications of Hypervalent Iodine Compounds
2016 Standout
The distribution of brominated long‐chain fatty acids in sponge and symbiont cell types from the tropical marine spongeAmphimedon terpenensis
1994
Impact of Natural Products on Developing New Anti-Cancer Agents
2009 Standout
Diplopuupehenone, a new unsymmetrical puupehenone-related dimer from the marine sponge Dysidea sp.
2011
Applications of Palladium-Catalyzed C–N Cross-Coupling Reactions
2016 Standout
Alkaloids from Marine Ascidians
2011
Cytotoxicity of Lissoclibadins and Lissoclinotoxins, Isolated from a Tropical Ascidian Lissoclinum cf. badium, against Human Solid-Tumor-Derived Cell Lines
2007
Hydroperoxysterols from the Tunicate Eudistoma sp.
2007
Transition-Metal-Catalyzed Reactions in Heterocyclic Synthesis
2004 Standout
Catalytic Asymmetric Intramolecular [4+2] Cycloaddition of In Situ Generated ortho‐Quinone Methides
2017 StandoutNobel
Lissoclinotoxins E and F, novel cytotoxic alkaloids from a Philippine didemnid ascidian
2003
Isolation and biological activity of (E)-1-(4-hydroxystyryl)guanidine from the sub-Arctic ascidian, Dendrodoa aggregata
2010
Phylogenetic Diversity of Bacteria Associated with the Marine Sponge Rhopaloeides odorabile
2001
Two New Ceramides from the Marine Sponge Ircinia fasciculata
2005
Small Peptides Catalyze Highly Enantioselective Direct Aldol Reactions of Aldehydes with Hydroxyacetone: Unprecedented Regiocontrol in Aqueous Media
2004
Purpurogemutantin and Purpurogemutantidin, New Drimenyl Cyclohexenone Derivatives Produced by a Mutant Obtained by Diethyl Sulfate Mutagenesis of a Marine-Derived Penicillium purpurogenum G59
2012
Additional Insights on the Bastadins: Isolation of Analogues from the Sponge Ianthella cf. reticulata and Exploration of the Oxime Configurations
2010
Steroid and cembranoids from the Dongsha atoll soft coral Lobophytum sarcophytoides
2010
Systems biology of cyanobacterial secondary metabolite production and its role in drug discovery
2008
Cytotoxic Isomalabaricane Triterpenes from the Marine Sponge Rhabdastrella globostellata
2006
Synthesis and determination of the relative structure of akaterpin, a potent inhibitor of PI-PLC
2011
Effects of Caribbean sponge secondary metabolites on bacterial surface colonization
2005
Gold-Catalyzed Carbon−Heteroatom Bond-Forming Reactions
2011 Standout
Polycyclische Aromatische Alkaloide, V. Synthese von 2‐Bromleptoclinidinon
1990
Aryne, ortho-Quinone Methide, and ortho-Quinodimethane: Synthesis of Multisubstituted Arenes Using the Aromatic Reactive Intermediates
2010
Synthesis of Biaryls via a Nickel(0)-Catalyzed Cross-Coupling Reaction of Chloroarenes with Arylboronic Acids
1997
Chemistry and Biology Of Multicomponent Reactions
2012 Standout
Isomalabaricane-Type Compounds from the Marine Sponge Rhabdastrella aff. distincta
2004
Dynamic kinetic resolution
1995
Determination of the Absolute Structure of (+)-Akaterpin
2012
Lophocladines, Bioactive Alkaloids from the Red Alga Lophocladia sp.
2006
Rhabdastrellins A−F, Isomalabaricane Triterpenes from the Marine Sponge Rhabdastrella aff. distincta
2008
Zorrimidazolone, a Bioactive Alkaloid from the Non-Indigenous Mediterranean Stolidobranch Polyandrocarpa zorritensis
2011
Planar Chirality due to a Polysulfur Ring in Natural Pentathiepin Cytotoxins. Implications of Planar Chirality for Enantiospecific Biosynthesis and Toxicity
2007
Total syntheses of the bromotyrosine-derived natural products ianthelline, 5-bromoverongamine and JBIR-44
2010
New Meroterpenoids from the Marine Sponge Aka coralliphaga
2012
Heterocyclic Nanographenes and Other Polycyclic Heteroaromatic Compounds: Synthetic Routes, Properties, and Applications
2016 Standout
Biosynthetic and Biomimetic Electrocyclizations
2005
Asymmetric Enamine Catalysis
2007 StandoutNobel
Lamellarins and Related Pyrrole-Derived Alkaloids from Marine Organisms
2007 Standout
Total Synthesis of (±)‐Dynemicin A
1995
New Scalarane-Based Sesterterpenes from the Sponge Phyllospongia madagascarensis
2004
The Marine Bromotyrosine Derivatives
2005
Isolation and Synthesis of Biologically Active Carbazole Alkaloids
2002 Standout
Aryl−Aryl Bond Formation One Century after the Discovery of the Ullmann Reaction
2002 Standout
Recent Advances in the Baylis−Hillman Reaction and Applications
2003 Standout
Anti-inflammatory Activity of a New Sphingosine Derivative and Cembrenoid Diterpene (Lobohedleolide) Isolated from Marine Soft Corals of Sinularia crassa TIXIER-DURIVAULT and Lobophytum species of the Andaman and Nicobar Islands
2005
Phenolic constituents of
1987
Novel Bromotyrosine Alkaloids: Inhibitors of Mycothiol S-Conjugate Amidase
2001
Xestospongienols A–L, Brominated Acetylenic Acids from the Chinese Marine Sponge Xestospongia testudinaria
2011
Gold(I)-Catalyzed Activation of Alkynes for the Construction of Molecular Complexity
2015 Standout
Cembrane Diterpenes Chemistry and Biological Properties
2012
Synthesis of 2,5‐Diaminoquinones by One‐Pot Copper‐Catalyzed Aerobic Oxidation of Hydroquinones and Addition Reaction of Amines
2009
Oxazinin-1, -2 and -3 − A Novel Toxic Compound and Its Analogues from the Digestive Glands ofMytilus galloprovincialis
2001
Cytotoxic Oxygenated Desmosterols of the Red Alga Galaxaura marginata
1996
Flexusines A and B and Epimukulol from the Soft Coral Sarcophyton flexuosum
2008
Works of Michèle Guyot being referenced
Mucronatine, a new N -methyl purine from the French mediterranean marine sponge Stryphnus mucronatus
2001
New ketosteroids from the red alga Hypnea musciformis
2002
16β-Hydroxy-5α-cholestane-3,6-dione, a novel cytotoxic oxysterol from the red alga Jania rubens
2000
Purification and Partial Identification of Novel Antimicrobial Protein from Marine Bacterium Pseudoalteromonas Species Strain X153
2004
Coscinosulfate, a CDC25 phosphatase inhibitor from the sponge Coscinoderma mathewsi
2001
Short synthesis of 16β-hydroxy-5α-cholestane-3,6-dione a novel cytotoxic marine oxysterol
2006
5,9,23‐Triacontatrienoic methyl ester, an elastase inhibitor from the marine sponge Chondrilla nucula
2002
12-epi-heteronemin : New sesterterpene from the marine sponge Hyrtios erecta
1994
An 3-indolyl-imidazol-4-one from the tunicate Dendrodoa grossularia.
1986
One-step Synthesis of Tyromycin A and Analogues
1998
Total Synthesis and Determination of the Absolute Configuration of Coscinosulfate. A New Selective Inhibitor of Cdc25 Protein Phosphatase
2001
Bioactive bromopolyacetylenes from the marine sponge Xestospongia testudinaria
1992
Ianthelline, un nouveau derive de lfl dibromo-3,5 tyrosine, isole de l'eponge ianthella ardis (bahamas)
1986
New cytotoxic isomalabaricane-type sesterterpenes from the New Caledonian marine sponge Rhabdastrella globostellata
2000
Biologically active quinone and hydroquinone sesquiterpenoids from the sponge smenospongia sp.
1989
Lutoside: an acyl-1-(acyl-6′-mannobiosyl)-3-glycerol isolated from the sponge-associated bacterium Micrococcus luteus
1997
Smenospongine: A cytotoxic and antimicrobial aminoquinone isolated from sp.
1987
Nouveau derive indolique du thiadiazole-1,2,4, isole d'un tunicier (Dendrodoa grossularia).
1980
New Sphingosines from the Marine Sponge Grayella cyatophora
2002
An antiplasmodial new (bis)indole alkaloid from the hard coral Tubastraea sp.
2009
A New Indole Alkaloid from the Marine Tunicate Dendrodoa grossularia
1998
Metabolites from the Sponge-Associated Bacterium Pseudomonas Species
1999
New Lipids from the Tunicate Cystodytes cf. dellechiajei, as PLA2 Inhibitors
2000
ChemInform Abstract: Biologically Active Sesterterpenes from a New Caledonian Marine Sponge Hyrtios sp.
1996
Revised Assignments of the13C NMR Spectra of Grossularine-1 and -2 Using 2D Heteronuclear1H-13C Correlations
1996
Synthetic studies on spongistatins: synthesis of the C29–C44 fragment
2000
Bioactive metabolites from marine invertebrates
1994
Typology of secondary cyanobacterial metabolites from minimum spanning tree analysis
2004
Efficient Total Synthesis of (−)-Ilimaquinone
1998
Smenoqualone a novel sesquiterpenoid from the marine sponge Smenospongia sp.
1992
A short entry into the pyrido[2,3-b]indole ring system. Synthesis of the tetracyclic segment of the marine antitumor agents: Grossularines-1 and -2
1993
New Bromoditerpenes from the Red Alga Sphaerococcus coronopifolius
2001
Lissoclinotoxins: Antibiotic polysulfur derivatives from the tunicate Lissoclinum perforatum. Revised structure of lissoclinotoxin A
1994
Grossularine-1 and grossularine-2, cytotoxic α-carbolines from the tunicate: Dendrodoa grossularia
1989
Novel alkaloids of the aaptamine class from an Indonesian marine sponge of the genus Xestospongia
2003
Synthesis of (−)-Hyatellaquinone and Revision of Absolute Configuration of Naturally Occurring (+)-Hyatellaquinone
1999
Araplysillins-I and-II: Biologically active dibromotyrosine derivatives from the spongePsammaplysilla arabica
1990
Trikendiol, an unusual red pigment from the sponge Trikentrion loeve, anti-HIV-1 metabolite
1994
Hydroperoxy-24 vinyl-24 cholesterol, nouvel hydroperoxyde naturel isole de deux tuniciers : phallusia mamillata et ciona intestinalis.
1982
An expeditious synthesis of structural analogs of the marine cytotoxic agents grossularines-1 and -2
1995
Total synthesis of maesanin and analogues
1998
Lissoclinotoxin A, an antibiotic 1,2,3-trithiane derivative from the tunicate Lissoclinum perforatum.
1991
Methanol Adduct of Puupehenone, a Biologically Active Derivative from the Marine Sponge Hyrtios Species
1999
Nouvelle methode de synthese d'acides homophtaliques et d'homophtalimides par voie arynique. Application a la synthese de la Melleine.
1973
Grossularine-1 and grossularine-2, alpha carbolines from Dendrodoa grossularia, as possible intercalative agents.
1987
Grossularine, a novel indole derivative from the marine tunicate, dendrodoa grossularia
1984
Functional Specialization of Stable and Dynamic Microtubules in Protein Traffic in WIF-B Cells
1998
Two new cembrane diterpenes from a Madagascan soft coral of the genus Sarcophyton
2002
Dipuupehedione, a cytotoxic new red dimer from a new caledonian marine sponge hyrtios sp
1996
A new β-carboline alkaloid isolated from the marine sponge Hyrtios erecta
1996
Occurrence of 9(11)-ussaturated sterol peroxides in tunicates.
1981
Metabolites from the sponge-associated bacterium Micrococcus luteus.
1998